That's a nice list of goodies.
I would document what you are actually getting with a sound level meter and a test cd with individual frequency bands, then you know how much and which specific frequencies you need to 'tame'.
meter, tripod mount, put it ear level at listening position.
I use this Test CD, tracks 9-38 are 1/3rd octave from 25hz to 25k
If you cannot find it for a reasonable price, write me a message about it.
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After charting what you are getting, you might find a different location and/or toe-in helps I'm a big fan of level controls, both my main speakers (electrovoice drivers from 1956) and office (ar-2ax from 1967) have two level controls. Adjust the mid to the woofer, adjust the tweeter to the mid (interactive and l/r together, it ain't easy). Like yours, the quality/character of the sound is determined, only the relative volume is altered. After that, the character of the sound can be altered in small ways as you suggest, but I would not go at it without documenting what's what.