. . . Timeless, the Hank Williams tribute CD, had some interesting covers by some great artists. (I bought that one for Cold Cold Heart covered by Lucinda Williams, but it also featured Bob Dylan, Johnny Cash, Sheryl Crow, Keb Mo, Beck, Mark Knophler with EmmyLou, Tom Petty, Keith Richards, Ryan Adams and Hank III.)
Oops. On edit, I see that the OP already picked Timeless, but I second that nomination.